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Influence of UV degradation of bioplastics on the amplification of mercury bioavailability in aquatic environments 1 1 Introduction 1 2 Materials and methods 2 2.1 Chemicals and reagents 2 2.2 Accelerated UV-aging 2 2.3 Characterization of BIO and PE films 2 2.3.1 Chemical profile 2 2.3.2 Water wettability 2 2.3.3 Thickness and tensile properties 2 2.3.4 Surface topography, electrophysical properties, and microstructure 2 2.4 Hg-sorption experiments 2 2.4.1 Sorption kinetics 3 2.5 Statistical analysis 3 3 Results 3 3.1 Influence of UV-aging on physicochemical and mechanical profile of BIO and PE films 3 3.2 Impact of UV-aging on the Hg-sorption performance of BIO and PE films 4 3.3 Influence of initial concentration and ionic strength on Hg-sorption performance of BIO and PE films 4 4 Discussion 5 4.1 Influence of accelerated aging in BIO and PE properties 5 4.2 Influence of UV-aging in Hg-sorption ability by BIO and PE films 6 4.3 Implication of the BIO plastic degradation in aquatic environments and subsequent interaction with Hg 7 5 Conclusions 9 CRediT authorship contribution statement 9 Declaration of competing interest 9 Acknowledgements 9 References 9

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UND

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nonfiction