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Thermally-Induced Structural Evolution of Silicon- and Oxygen-Containing Hydrogenated Amorphous Carbon by Mangolini, Filippo; Hilbert, James; McClimon, J. Brandon; Lukes, Jennifer R.; Carpick, Robert W. is a scholarly article available to read on EtoBox.

What is Thermally-Induced Structural Evolution of Silicon- and Oxygen-Containing Hydrogenated Amorphous Carbon about?

The thermally-induced structural evolution of silicon- and oxygen-containing hydrogenated amorphous carbon (a-C:H:Si:O) was investigated by X-ray photoelectron and absorption spectroscopy, as well as molecular dynamics (MD) simulations. The spectroscopic results indicate that the introduction of Si and O in hydrogenated amorphous carbon (a-C:H) increases the activation energy for the conversion of sp3- to sp2-bonded C. MD simulations indicate that the higher thermal stability of a-C:H:Si:O compared to a-C:H derives from the lower fraction of strained C-C sp3 bonds in a-C:H:Si:O.

Author

Mangolini, Filippo; Hilbert, James; McClimon, J. Brandon; Lukes, Jennifer R.; Carpick, Robert W.

Published

2017

Language

EN