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This document summarizes a study on improving the electrocatalytic CO2 reduction activity and selectivity of a Fe-porphyrin-based metal–organic framework (MOF) by introducing electrostatic secondary-sphere interactions. The researchers found that immobilizing positively-charged groups near the Fe catalyst in the MOF stabilized reactive CO intermediates, allowing their rapid release and improving CO production. They also showed systematic control of electrostatic field strength by varying electrolyte concent

Author

pandiaraj1988

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EN