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Coherent Spin Dynamics of Electrons in Two-Dimensional (PEA)$ 2$PbI$ 4$ Perovskites by Kirstein, Erik; Zhukov, Evgeny A.; Yakovlev, Dmitri R.; Kopteva, Nataliia E.; Harkort, Carolin; Kudlacik, Dennis; Hordiichuk, Oleh; Kovalenko, Maksym V.; Bayer, Manfred is a scholarly article available to read on EtoBox.

What is Coherent Spin Dynamics of Electrons in Two-Dimensional (PEA)$ 2$PbI$ 4$ Perovskites about?

The versatile potential of lead halide perovskites and two-dimensional materials is merged in the Ruddlesen-Popper perovskites having outstanding optical properties. Here, the coherent spin dynamics in Ruddlesen-Popper (PEA)$_2$PbI$_4$ perovskites are investigated by picosecond pump-probe Kerr rotation in an external magnetic field. The Larmor spin precession of resident electrons with a spin dephasing time of 190~ps is identified. The longitudinal spin relaxation time in weak magnetic fields measured by the spin inertia method is as long as 25~$\mu$s. A significant anisotropy of the electron $g$-factor with the in-plane value of $+2.45$ and out-of-plane value of $+2.05$ is found. The exciton out-of-plane $g$-factor is measured to be of $+1.6$ by magneto-reflectivity. This work contributes to the understanding of the spin-dependent properties of two-dimensional perovskites and their spin dynamics.

Author

Kirstein, Erik; Zhukov, Evgeny A.; Yakovlev, Dmitri R.; Kopteva, Nataliia E.; Harkort, Carolin; Kudlacik, Dennis; Hordiichuk, Oleh; Kovalenko, Maksym V.; Bayer, Manfred

Published

2022

Language

EN