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POLYCRYSTALLINE AND SPATIALLY NON-HOMOGENEOUS AMORPHOUS SEMICONDUCTORS AND INSULATORS 3 POLYCRYSTALLINE AND SPATIALLY NON-HOMOGENEOUS AMORPHOUS SEMICONDUCTORS AND INSULATORS 5 NOTICE TO THE READER 6 CONTENTS 7 ABSTRACT 11 PREFACE 15 ACKNOWLEDGMENTS 29 Chapter 1: INTRODUCTION AND HISTORICAL BACKGROUND 31 1.1. DENSITY OF ELECTRON SATES IN POLYCRYSTALLINE AND AMORPHOUS SEMICONDUCTORS: STANDARD MODELS 34 1.2. PHONON CONFINEMENT PHENOMENON AND CORRELATION LENGTH OF DISORDER 42 1.3. MORPHOLOGY, LONG RANGE POTENTIAL FLUCTUATIONS, AND PROPERTIES OF A-SI:H 44 1.4. MORPHOLOGY, CHEMICAL COMPOSITION, STRUCTURAL, OPTICAL AND BAND TAIL PARAMETERS OF POROUS AMORPHOUS LOW-K DIELECTRIC THIN FILMS AND POROUS SILICON 47 1.5. MORPHOLOGY, ELECTRON SPECTRUM AND MACROSCOPIC PROPERTIES OF STRAINED CRYSTALLINE SILICON, GERMANIUM AND SILICON-GERMANIUM LAYERS 52 1.6. MORPHOLOGY, STRUCTURAL DISORDER, PHONON CONFINEMENT, AND NEAR-BAND-GAP OPTICAL ABSORPTION OF POLYCRYSTALLINE DIAMOND 60 Chapter 2: GENERALIZED SKETTRUP MODEL FOR DENSITY OF ELECTRON STATES IN POLYCRYSTALLINE SEMICONDUCTORS 67 2.1. PHONON FLUCTUATIONS AND ELECTRON LEVELS IN SOLIDS 67 2.2. GENERALIZED SKETTRUP MODEL (GSM) 71 2.3. SIMULATION PARAME

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