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The precision-complexity binomial to achieve the best mathematical-thermodynamic modelling on the Gibbs-function and its effect on the separation processes design 1 Introduction 1 The global working approach 2 Thermodynamic formalism 4 Parameterization procedure 6 Multiproperty modelling and control of complexity 6 Formulation of the multiobjective problem 7 Resolution method 8 Results of the modelling 9 Analysis of the efficient-fronts 9 Model performance analysis 10 Description of the volumetric behaviour 11 Feasibility of ester purification from a solution of butyl butanoate + decane 12 Conclusions 16 Declaration of Competing Interest 18 Acknowledgements 18 Appendix A A procedure based on Tait equation to describe the p-rho-T behaviour of pure compounds 18 Appendix B &gulliverv;E error decoupling from VLEs and hEs 18 Appendix C Method for generating a random initial population for the genetic algorithm 19 Appendix D Supplementary data 20 References 20
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