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Femtosecond Raman-induced polarization spectroscopy studies of rotational coherence in O2, N2 and CO2 by M. Morgen; W. Price; L. Hunziker; P. Ludowise; M. Blackwell; Y. Chen is a Physics and Astronomy article available to read on EtoBox.

What is Femtosecond Raman-induced polarization spectroscopy studies of rotational coherence in O2, N2 and CO2 about?

Using the femtosecond Raman-induced polarization spectroscopy (RIPS) technique, we have observed ground vibronic state rotational coherence in gaseous N2, COZ and OZ. Both theoretical and experimental studies are reported. The theory is in excellent agreement with experiment. At earlier pump-probe delays, the time evolution of the polarization recurrence is well described by a rigid rotor model. Higher order spectroscopic constants are extracted from longer delay time spectra. The rotational relaxation constants for ground vibmnic state N2 and 02 are also measured using the real-time technique.

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Author

M. Morgen; W. Price; L. Hunziker; P. Ludowise; M. Blackwell; Y. Chen

Publisher

Elsevier Science; Elsevier ; Elsevier BV (ISSN 0009-2614)

Published

1993

Language

EN

Field

Physics and Astronomy (Physical Sciences)