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Ultrafast Hot Electron Dynamics in Plasmonic Nanostructures: Experiments, Modelling, Design by Andrea Schirato; Margherita Maiuri; Giulio Cerullo; Giuseppe Della Valle is a scholarly article available to read on EtoBox.

What is Ultrafast Hot Electron Dynamics in Plasmonic Nanostructures: Experiments, Modelling, Design about?

Abstract Metallic nanostructures exhibit localized surface plasmons (LSPs), which offer unprecedented opportunities for advanced photonic materials and devices. Following resonant photoexcitation, LSPs quickly dephase, giving rise to a distribution of energetic ‘hot’ electrons in the metal. These out-of-equilibrium carriers undergo ultrafast internal relaxation processes, nowadays pivotal in a variety of applications, from photodetection and sensing to the driving of photochemical reactions and ultrafast all-optical modulation of light. Despite the intense research activity, exploitation of hot carriers for real-world nanophotonic devices remains extremely challenging. This is due to the complexity inherent to hot carrier relaxation phenomena at the nanoscale, involving short-lived out-of-equilibrium electronic states over a very broad range of energies, in interaction with thermal electronic and phononic baths. These issues call for a comprehensive understanding of ultrafast hot electron dynamics in plasmonic nanostructures. This paper aims to review our contribution to the field: starting from the fundamental physics of plasmonic nanostructures, we first describe the experimental

Author
Andrea Schirato; Margherita Maiuri; Giulio Cerullo; Giuseppe Della Valle
Publisher
Walter de Gruyter GmbH
Published
2023
Language
EN