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The study investigates the chlorination reaction behavior of Zircaloy-4 hull waste using HSC chemistry code, focusing on the impact of decladding ratio on the reaction. The simulation suggests that solid phase chlorides are produced before the formation of ZrCl4(g), which can be easily separated due to its gaseous state at 330 °C. The findings indicate that the chlorination method could effectively recover highly pure ZrCl4 from hull waste, potentially reducing the volume and cost of high-level waste manage

Author

Francis Muliangala

Language

EN