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Fundamentals and practical dielectric implications of stoichiometry and chemical design in a high-performance ferroelectric ... 1 1 Brief history of BaTiO3 and its technological importance 1 2 Defect chemistry, crystal chemistry, and selected property fundamentals of BaTiO3 2 3 Phase equilibria and its relationship to defect chemistry of BaTiO3 4 4 Doping strategies and types in BaTiO3 6 4.1 Isovalent doping 7 4.2 Aliovalent doping 7 4.2.1 Donor doping 7 4.2.2 Acceptor doping 7 4.2.3 Amphoteric doping 7 4.2.4 Co-doping strategies 8 4.2.5 Defect complexes 8 4.2.6 Defects at surfaces and grain boundaries 10 5 Modeling defect energetics and properties 10 6 Bulk conduction mechanisms 10 6.1 Conduction in polycrystalline BaTiO3 ceramics 12 6.1.1 Electrode n-type BaTiO3 interface cases 12 6.1.2 Grain boundary interfaces 13 7 Examples of defect dynamics under temperature and electric fields in BaTiO3 related materials 14 7.1 Association-dissociation of oxygen vacancies in defect complexes 14 7.2 Ferroelectric aging 15 7.3 Polarization switching fatigue in Ferroelectrics 16 7.4 Colossal permittivity 17 7.5 Electromigration and resistance degradation 17 8 Capacitive BaTiO3 based application

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