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Enabling resource circularity through thermo-catalytic and solvent-based conversion of waste plastics 1 Introduction 1 Hydroconversion 5 Polyolefins 6 Pt catalysts 6 Zr catalysts 11 Ru catalysts 12 Polyesters 14 Mechanistic insights from model compounds and plastics hydroconversion 16 Model compound hydrogenolysis 17 Polymer hydrogenolysis 17 Degree of substitution in hydrogenolysis 18 Hydrocracking 19 Solvolytic conversion 20 Solvolysis 20 Polyesters 20 Polycarbonates 23 Tandem solvolysis and catalysis 23 Polyesters 24 Polycarbonates 25 Solvent extraction 26 Catalytic conversion without solvents or gaseous reagents 27 Challenges and opportunities 29 Experimental standardization 29 Reaction conditions and parameters 30 Catalyst design, characterization, and modeling 31 Product selectivity and yield 31 Process design 31 Conclusions and outlook 33 Supplemental information 33 Acknowledgments 33 Author contributions 33 Declaration of interests 33 References 33
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Common subject areas: history, science, philosophy, social sciences.
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- nonfiction