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Infrared Photodissociation Spectroscopy of Mass-Selected Cu 2 O 2 (CO) n + Clusters in the Gas Phase by Xin, Ke; Chen, Yinjuan; Zhang, Luning; Wang, Xuefeng; Wang, Guanjun is a Chemistry article available to read on EtoBox.

What is Infrared Photodissociation Spectroscopy of Mass-Selected Cu 2 O 2 (CO) n + Clusters in the Gas Phase about?

The stoichiometric Cu 2 O 2 (CO) n + (n = 3-7) clusters are generated via a laser vaporization supersonic cluster source in gas phase and identified by infrared photodissociation spectroscopy in the C-O stretching region. The infrared spectra are interpreted and the cluster structures are determined by density functional calculations. The ground state of Cu 2 O 2 (CO) n + are intrinsically a dicopper superoxide carbonyl with [(OC) x CuOOCu(CO) y ] + ( x + y = n) structures in which CO ligands coordinate a zigzag Cu(OO)Cu + core. The structure characterization for Cu(OO)Cu + core-based clusters is crucial to correctly understand the associated catalytic reactions by metal clusters.

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Author

Xin, Ke; Chen, Yinjuan; Zhang, Luning; Wang, Xuefeng; Wang, Guanjun

Publisher

American Chemical Society; American Chemical Society (ACS) (ISSN 1089-5639)

Published

2020

Language

EN

Field

Chemistry (Physical Sciences)