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This study investigates the structural transformations of Rh particles in Rh ion-exchanged zeolite (RhY) and Li-doped RhY (Li/RhY) during CO2 hydrogenation. The findings reveal that while RhY primarily produces methane, the addition of Li alters the reaction pathway to favor CO production, with distinct dynamic structures observed via EXAFS analysis. The research proposes a new mechanism for catalysis influenced by the presence of Li, highlighting its significant effect on the reactivity of Rh catalysts.

Author

zayhalvid

Language

EN