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Interpretation of Multidimensional Coherent Spectra by Hebin Li; Bachana Lomsadze; Galan Moody; Christopher L. Smallwood; Steven T. Cundiff is a book available to read on EtoBox.

What is Interpretation of Multidimensional Coherent Spectra about?

Abstract Interpretation of multi-dimensional coherent spectra is presented in this chapter. Results are presented with the Bloch model. We begin by discussing the characteristic features of an MDCS rephasing plot corresponding to a two-level system. We then discuss the characteristics of inhomogeneous ensembles of two-level systems. We go on to discuss the origins of cross-peaks in MDCS, and then some of the signatures in MDCS that arise as a result of many-body effects. Double-quantum spectra, zero-quantum spectra, three-dimensional spectra, and nonrephasing single-quantum spectra are discussed. Finally, we discuss the impact that finite pulse effects can have on a multidimensional spectrum.

Author

Hebin Li; Bachana Lomsadze; Galan Moody; Christopher L. Smallwood; Steven T. Cundiff

Publisher

Oxford University PressOxford

Published

2023

Language

EN

ISBN

9780192843869

Subjects

Science, Chemistry, Physics