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The Role of Defects in Metal–Organic Frameworks for Nitrogen Reduction Reaction: When Defects Switch to Features by Islam E. Khalil; Cong Xue; Wenjing Liu; Xiaohan Li; Yu Shen; Sheng Li; Weina Zhang; Fengwei Huo is a Engineering article available to read on EtoBox.

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## Abstract The electrochemical nitrogen reduction reaction (NRR), a contributor for producing ammonia under mild conditions sustainably, has recently attracted global research attention. Thus far, the design of highly efficient electrocatalysts to enhance NRR efficiency is a specific focus of the research. Among them, defect engineering of electrocatalysts is considered a significant way to improve electrocatalytic efficiency by regulating the electronic state and providing more active sites that can give electrocatalysts better physicochemical properties. Recently, metal–organic frameworks (MOFs), along with their derivatives, have captured immense interest in electrocatalytic reactions owing to not only their large surface area and high porosity but also the ability to create rich defects in their structures. Hence, they can provide plenty of exposed active sites for electron transfer, NN cleavage, and N~2~ adsorption to enhance NRR performance. Herein, the concept, the in situ characterizations techniques for defects, and the most common ways to create defects into MOFs have been summarized. Furthermore, the recent advances of MOF‐based electrocatalysts towards NRR have been r

Who reads The Role of Defects in Metal–Organic Frameworks for Nitrogen Reduction Reaction: When Defects Switch to Features?

Author

Islam E. Khalil; Cong Xue; Wenjing Liu; Xiaohan Li; Yu Shen; Sheng Li; Weina Zhang; Fengwei Huo

Publisher

Wiley

Published

2021

Language

EN

Field

Engineering (Physical Sciences)