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This study presents a novel method for fabricating highly oriented ultrathin zirconium metal-organic framework (Zr-MOF) membranes, specifically UiO-66, using anisotropic etching and epitaxial growth techniques. The resulting membranes demonstrate exceptional gas separation performance, achieving unprecedented CO2 permeance and selectivity compared to existing polycrystalline MOF membranes. The research highlights the importance of microstructural control in enhancing the efficiency of membrane-based gas sep

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liruiying1126

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EN