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Magnetic properties of frustrated spin-$\frac{1}{2}$ capped-kagome antiferromagnet (CsBr)Cu$ 5$V$ 2$O$ {10}$ by Guchhait, S.; Ambika, D. V.; Mohanty, S.; Furukawa, Y.; Nath, R. is a scholarly article available to read on EtoBox.

What is Magnetic properties of frustrated spin-$\frac{1}{2}$ capped-kagome antiferromagnet (CsBr)Cu$ 5$V$ 2$O$ {10}$ about?

The structural and magnetic properties of a spin-$\frac{1}{2}$ averievite (CsBr)Cu$_5$V$_2$O$_{10}$ are investigated by means of temperature-dependent x-ray diffraction, magnetization, heat capacity, and $^{51}$V nuclear magnetic resonance (NMR) measurements. The crystal structure (trigonal, $P\bar{3}$) features a frustrated capped-kagome lattice of the magnetic Cu$^{2+}$ ions. Magnetic susceptibility analysis indicates a large Curie-Weiss temperature of $\theta_{\rm CW} \simeq-175$ K. Heat capacity signals the onset of a magnetic long-range-order (LRO) at $T_{\rm N}\simeq 21.5$ K at zero magnetic field due to the presence of significant inter-planer coupling in this system. The magnetic LRO below 27 K is further evident from the drastic change in the $^{51}$V NMR signal intensity and rapid enhancement in the $^{51}$V spin-lattice relaxation rate in a magnetic field of 6.3 T. The frustration index $f=|\theta_{\rm CW}|/T_{\rm N} \simeq 8$ ascertains strong magnetic frustration in this compound. From the high-temperature value of the $^{51}$V NMR spin-lattice relaxation rate, the leading antiferromagnetic exchange interaction between the Cu$^{2+}$ ions is calculated to be $J/k_{\rm B

Author

Guchhait, S.; Ambika, D. V.; Mohanty, S.; Furukawa, Y.; Nath, R.

Published

2024

Language

EN