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This study investigates the mechanism of directed lithiations through the analysis of intra- and intermolecular kinetic isotope effects for specific substrates. The findings suggest a two-step mechanism involving initial complexation followed by hydrogen transfer, particularly for the lithiation of N-benzyl-N,N′-dimethyl urea and amides. The results provide insights into the role of complex-induced proximity effects in enhancing the efficiency of lithiation reactions.

Author

valeriverhov

Language

EN