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Photocatalytic Activity of Graphene Oxide/zinc Oxide Nanocomposite Derived from Rice Husk for the Degradation of Phenanthrene Under Ultraviolet-visible Light by Husn Ara Chauhan; Mohd Rafatullah; Khozema Ahmed Ali; Mohammad Faisal Umar; Moonis Ali Khan; Byong-Hun Jeon is a Environmental Science article available to read on EtoBox.

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Environmental concerns have arisen due to the persistent nature and carcinogenicity of polycyclic aromatic hydrocarbons (PAHs). This study used the doping approach to successfully develop a nanocomposite photocatalyst based on graphene oxide (GO) and zinc oxide (ZnO). The nanocomposites were investigated by Fourier transform infrared (FTIR) spectroscopy, UV-Visible diffuse reflectance spectroscopy (UV-Vis DRS), x-ray diffraction (XRD), scanning electron microscopy (SEM) with energy dispersive x-ray (EDX), transmission electron microscopy (TEM), Brunauer-Emmett-Teller (BET), and Raman spectroscopy. GO/ZnO nanocomposite showed excellent ability to degrade 25 ppm of phenanthrene (86.06%) in 120 min under UV-Visible light exposure followed by photolysis (no photocatalyst) (15.56%), GO/ZnO without stirring (40.28%), GO/ZnO in the dark with stirring (47.40%), and commercial ZnO (62.84%). This is due to the largest surface area, which was enhanced by the doping of GO in commercial ZnO. Phenanthrene photodegradation by GO/ZnO nanocomposite followed first-order kinetics with a rate constant of 0.0375 min -1 . The smaller byproducts like (Z)-3-hydroxy acrylic acid (1b; m/z = 88) and (Z)-4-ox

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Author

Husn Ara Chauhan; Mohd Rafatullah; Khozema Ahmed Ali; Mohammad Faisal Umar; Moonis Ali Khan; Byong-Hun Jeon

Publisher

Elsevier BV

Published

2022

Language

EN

Field

Environmental Science (Physical Sciences)