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Bimetallic Fe/Ti‐Based Metal–Organic Framework for Persulfate‐Assisted Visible Light Photocatalytic Degradation of Orange II by Minghua Wang; Longyu Yang; Chuanpan Guo; Xufei Liu; Linghao He; Yingpan Song; Qingxin Zhang; Xiongwei Qu; Hongzhong Zhang; Zhihong Zhang; Shaoming Fang is a Chemistry article available to read on EtoBox.
What is Bimetallic Fe/Ti‐Based Metal–Organic Framework for Persulfate‐Assisted Visible Light Photocatalytic Degradation of Orange II about?
## Abstract Amine‐functionalized bimetallic Fe/Ti‐based metal–organic frameworks (Fe/Ti‐MOF‐NH~2~) were synthesized via the solvothermal method and used as photocatalysts and activators for persulfate (PS)‐assisted visible light photocatalytic degradation of Orange II. Nearly 100% of Orange II was removed within 10 min in the Fe/Ti‐MOF‐NH~2~(3:1)/PS/Vis process, while only 10.7% and 70.9% of Orange II were removed in Fe/Ti‐MOF‐NH~2~(3:1)/Vis and Fe/Ti‐MOF‐NH~2~(3:1)/PS processes within 10 min, respectively. Therefore, the synergistic effect of PS activation and visible light photocatalysis was demonstrated by the Fe/Ti‐MOF‐NH~2~(3:1) composite. The enhanced photocatalytic activity of the photocatalyst can be attributed to the efficient electrons transfer by Fe^3+^/Fe^2+^ and Ti^4+^/Ti^3+^ redox cycles, activation of PS by photogenerated electrons to produce sulfate radicals (SO~4~^•−^), and increased formation of hydroxyl radicals (^•^OH). Concurrently, the Fe/Ti‐MOF‐NH~2~(3:1) photocatalyst also exhibited good reusability and stability in the photocatalytic reaction system.
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- Author
- Minghua Wang; Longyu Yang; Chuanpan Guo; Xufei Liu; Linghao He; Yingpan Song; Qingxin Zhang; Xiongwei Qu; Hongzhong Zhang; Zhihong Zhang; Shaoming Fang
- Publisher
- Wiley
- Published
- 2018
- Language
- EN
- Field
- Chemistry (Physical Sciences)