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The document discusses the synthesis and characterization of a diiron dithiolate complex, (μ-S)2Fe2(CO)6, which is covalently embedded in a β-barrel protein matrix to function as an artificial hydrogenase. This hybrid catalyst demonstrates significant photocatalytic activity for hydrogen evolution, achieving a turnover number of up to 130 in the presence of a Ru photosensitizer and ascorbate. The study highlights the potential of integrating synthetic metal complexes within protein scaffolds to enhance cata

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linlimeee

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EN