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Hyperspherical modes by J. Manz; H.H.R. Schor is a Physics and Astronomy article available to read on EtoBox.
What is Hyperspherical modes about?
Hyperspherk! zlodes for bound and resonance states of linear ABA molecules are predicted um a Morse-oscillator model. These modes oscillate approximately along circles with constant hyperspherical radius. Prominent hyperspherical modes should occur in dihydrides with exclusive excitation of the antisymmetric stretching mode IJ~ > 0. l\_ Introduction A molecule may store excitation energy in various types of vrbrational states. Those most studied are the normal and local modes [l-17]. These regular modes co-exist in a narrow energy range even if they describe complerely different molecular oscillations, e.g. smalland large-amplitude motions of large molecular fragments and individual bonds, respectively. Experimentally, the co-existence of different modes implies the selectivity of a large variety of molecular properties, including electromagnetic moments, rotational constants and reactivity. Clearly, it is important to understand the nature of excited virbrational states. In this paper, we suggest a third class of regular vibrations: hyperspherical modes. They also co-exist with normal and local modes. Normal modes oscillate along normal coordinates centered at the minimum of the p
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- Author
- J. Manz; H.H.R. Schor
- Publisher
- Elsevier Science; Elsevier ; Elsevier BV (ISSN 0009-2614)
- Published
- 1984
- Language
- EN
- Field
- Physics and Astronomy (Physical Sciences)