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Can I read Very low-pressure pyrolysis (VLPP) of 3,3-dimethylbut-1-yne (tert-butyl acetylene). The heat of formation and stabilization energy of the dimethylpropargyl radical on EtoBox?

Very low-pressure pyrolysis (VLPP) of 3,3-dimethylbut-1-yne (tert-butyl acetylene). The heat of formation and stabilization energy of the dimethylpropargyl radical by Keith D. King is a Chemistry article available to read on EtoBox.

What is Very low-pressure pyrolysis (VLPP) of 3,3-dimethylbut-1-yne (tert-butyl acetylene). The heat of formation and stabilization energy of the dimethylpropargyl radical about?

The unimolecular decomposition of 3,3-dimethylbut-l-yne has been investigated over the temperature range of 933"-1182"K using the technique of very low-pressure pyrolysis (VLPP). The primary process is C-C bond fission yielding the resonance stabilized dimethylpropargyl radical. Application of RRKM theory shows that the experimental unimolecular rate constants are consistent with the high-pressure Arrhenius parameters given by log (klsec-l) = (15.8 f 0.3) -(70.8 f 1.5)/8 where 8 = 2.303RT kcal/mol. The activation energy leads to DH0[(CH&C(CCH)-CH3] = 70.7 f 1.5, AHP((CH&$CCHg) = 61.5 f 2.0, and DHO[(CH&C(CCH)-H] = 81.0 f 2.3, all in kcal/mol at 298°K. The stabilization energy of the dimethylpropargyl radical has been found to he 11.0 f 2.5 kcal/mol.

Who reads Very low-pressure pyrolysis (VLPP) of 3,3-dimethylbut-1-yne (tert-butyl acetylene). The heat of formation and stabilization energy of the dimethylpropargyl radical?

It is typically read by researchers, students, and practitioners in Chemistry.

Author
Keith D. King
Publisher
John Wiley and Sons; Wiley (John Wiley & Sons); John Wiley & Sons Inc.; Wiley (ISSN 0538-8066)
Published
1977
Language
EN
Field
Chemistry (Physical Sciences)

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