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Impedance spectra of porous, composite intercalation electrodes: The origin of the low-frequency semicircles by M.D. Levi; D. Aurbach is a Engineering article available to read on EtoBox.

What is Impedance spectra of porous, composite intercalation electrodes: The origin of the low-frequency semicircles about?

Impedance spectra of composite, graphite electrodes, which are highly porous with a poor orientation of their particles show well-developed low-frequency semicircles (LFSs) with formally very high characteristic capacitances (about 160 mF cm -2 ), which cannot be rationalized on the basis of the porous electrodes models known from the literature. We use herein a new model (recently reported in full detail) considering two (or more) porous sublayers of different thicknesses, which readily reproduces the well-developed LFSs with very high characteristic capacitances (C LFS in the range from 0.05 to 5 F cm -2 using typical values of electrodes parameters, calculated from ω max ). A detailed analysis shows that the LFSs characterizing the impedance spectra of highly porous graphite electrodes, have a simple "geometric" meaning. They result from a parallel combination of the intercalation capacitance of the thinnest sublayer and the high, active resistance of the thicker layer.

Who reads Impedance spectra of porous, composite intercalation electrodes: The origin of the low-frequency semicircles?

It is typically read by researchers, students, and practitioners in Engineering.

Author
M.D. Levi; D. Aurbach
Publisher
Elsevier Science; Elsevier ; Elsevier BV (ISSN 0378-7753)
Published
2005
Language
EN
Field
Engineering (Physical Sciences)

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