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Photodissociation dynamics of OCS and CS2 adsorbed on water ice films at 193 nm by Atsushi Ikeda; Noboru Kawanaka; Akihiro Yabushita; Masahiro Kawasaki is a Materials Science article available to read on EtoBox.

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Photodissociation dynamics of OCS and CS 2 adsorbed on water ice films at 90 K was investigated at 193 nm by measuring the time-of-flight spectra of photodissociated S( 1 D) and S( 3 P) atoms. The translational energy distributions are well represented by a combination of Gaussian and Maxwell-Boltzmann (M-B) distributions corresponding to the fast and slow time-of-flight components, respectively. Formation of the sulfur dimer on the ice surface is proposed as a secondary photoproduct. The fine-structure branching ratios of S( 3 P J ) from OCS and CS 2 adsorbed on H 2 O or D 2 O water ice films were also determined.

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Author

Atsushi Ikeda; Noboru Kawanaka; Akihiro Yabushita; Masahiro Kawasaki

Publisher

Elsevier Science; Elsevier ; Elsevier BV (ISSN 1010-6030)

Published

2008

Language

EN

Field

Materials Science (Physical Sciences)