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Optimization of process parameters and catalyst compositions in carbon dioxide oxidative coupling of methane over CaO–MnO/CeO2 catalyst using response surface methodology by Istadi; Nor Aishah Saidina Amin is a Engineering article available to read on EtoBox.

What is Optimization of process parameters and catalyst compositions in carbon dioxide oxidative coupling of methane over CaO–MnO/CeO2 catalyst using response surface methodology about?

The optimization of process parameters and catalyst compositions for the CO 2 oxidative coupling of methane (CO 2 -OCM) reaction over CaO -MnO/CeO 2 catalyst was developed using Response Surface Methodology (RSM). The relationship between the responses, i.e. CH 4 conversion, C 2 hydrocarbons selectivity or yield, with four independent variables, i.e. CO 2 /CH 4 ratio, reactor temperature, wt.% CaO and wt.% MnO in the catalyst, were presented as empirical mathematical models. The maximum C 2 hydrocarbons selectivity and yields of 82.62% and 3.93%, respectively, were achieved by the individual-response optimization at the corresponding optimal process parameters and catalyst compositions. However, the CH 4 conversion was a saddle function and did not show a unique optimum as revealed by the canonical analysis. Moreover pertaining to simultaneous multi-responses optimization, the maximum C 2 selectivity and yield of 76.56% and 3.74%, respectively, were obtained at a unique optimal process parameters and catalyst compositions. It may be deduced that both individual-and multi-responses optimizations are useful for the recommendation of optimal process parameters and catalyst composition

Who reads Optimization of process parameters and catalyst compositions in carbon dioxide oxidative coupling of methane over CaO–MnO/CeO2 catalyst using response surface methodology?

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Author
Istadi; Nor Aishah Saidina Amin
Publisher
Elsevier Science; Elsevier ; Elsevier BV (ISSN 0378-3820)
Published
2006
Language
EN
Field
Engineering (Physical Sciences)

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