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This study investigates the coupling of redox and acid-base equilibria in ultrathin polyelectrolyte films, specifically a layer of poly(allylamine) with an osmium complex on a modified gold surface. Theoretical predictions indicate strong coupling effects at low ionic strength and near the pKa of the polyelectrolyte, which align with experimental observations from cyclic voltammetry. The findings suggest that the properties of the film, including thickness and protonation states, are influenced by pH and io

Author

mario.tagliazucchi

Language

EN