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Vibrational Energy Relaxation Pathways of Water by Andrei Pakoulev; Zhaohui Wang; Yoonsoo Pang; Dana D. Dlott is a Physics and Astronomy article available to read on EtoBox.

What is Vibrational Energy Relaxation Pathways of Water about?

Vibrational energy relaxation (VR) of the OH stretch m OH and bend d H 2 O in water is studied by the mid-IR pump with anti-Stokes Raman probe technique. The broad m OH band in water consists of two inhomogeneously broadened subbands. VR in the larger red-shifted subband m R OH , with T 1 1⁄4 0:55 ps, is shown to occur by the mechanism m OH ! d H 2 O (1/3) and m OH ! ground state (2/3). VR in the smaller longer-lived blue-shifted subband m B OH , with T 1 1⁄4 0:75 ps, occurs by the mechanism m OH ! ground state. The bending fundamental d H 2 O decays directly to the ground state with T 1 1⁄4 1:4 ps.

Who reads Vibrational Energy Relaxation Pathways of Water?

Author

Andrei Pakoulev; Zhaohui Wang; Yoonsoo Pang; Dana D. Dlott

Publisher

Elsevier Science; Elsevier ; Elsevier BV (ISSN 0009-2614)

Published

2003

Language

EN

Field

Physics and Astronomy (Physical Sciences)